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• W2740359760 abstract "Copolymer properties and processability depend on copolymer microstructure, i.e., copolymer composition and monomer unit arrangements along the copolymer chains. To predict the ultimate properties of copolymers, one needs complete information on the length and position of sequences of each monomer type in every chain. A versatile kinetic Monte Carlo code is developed and applied for the simulation of typical free radical copolymerizations. The code allows explicit monitoring of every growing chain during the course and at the end of polymerization, can account for comonomer systems of any arbitrary reactivity ratios ( r 1 and r 2 ) over the full range of monomer composition. Meanwhile, it eliminates the need for solving arrays of differential equations arising from deterministic modeling approaches. Since the code virtually synthesizes billions of copolymer molecules and keeps in storage information on each and every copolymer chain in the system, it allows for detailed statistical analysis. The simulator visualizes the bivariate sequence length–chain length distribution for typical copolymerization systems and examples with: r 1 < 1 and r 2 < 1; r 1 > 1 and r 2 < 1; ( r 1 × r 2 ) = 1; and r 1 = r 2 = 1, and is also applied successfully to an experimental scenario described in the literature." @default.
• W2740359760 created "2017-08-08" @default.
• W2740359760 creator A5005470736 @default.
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• W2740359760 date "2017-08-01" @default.
• W2740359760 modified "2023-10-16" @default.
• W2740359760 title "Visualization of Bivariate Sequence Length-Chain Length Distribution in Free Radical Copolymerization" @default.
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• W2740359760 doi "https://doi.org/10.1002/mats.201700041" @default.
• W2740359760 hasPublicationYear "2017" @default.
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