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• W2742459830 abstract "Stacking of disk-shaped organic molecules is a promising strategy to develop electronic and photovoltaic devices. Here, we investigate the capability of a soft block copolymer matrix that microphase separates into a cylindrical phase to direct the self-assembly of disk-shaped molecules by means of molecular simulations. We show that two disk molecules confined in the cylinder domain experience a depletion force, induced by the polymer chains, which results in the formation of stacks of disks. This entropic interaction and the soft confinement provided by the matrix are both responsible for the structures that can be self-assembled, which include slanted or columnar stacks. In addition, we evidence the transmission of stresses between the different minority domains of the microphase, which results in the establishment of a long-ranged interaction between disk molecules embedded in different domains; this interaction is of the order of the microphase periodicity and may be exploited to direct assembly of disks at larger scales." @default.
• W2742459830 created "2017-08-17" @default.
• W2742459830 creator A5006707355 @default.
• W2742459830 creator A5067179538 @default.
• W2742459830 date "2017-08-07" @default.
• W2742459830 modified "2023-09-27" @default.
• W2742459830 title "Block copolymer templated self-assembly of disk-shaped molecules" @default.
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• W2742459830 doi "https://doi.org/10.1063/1.4993210" @default.
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