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- W2743139035 abstract "The effect of molecule-molecule interactions on the size and shape of two-dimensional (2-D) ordering domains was investigated using scanning tunneling microscopy (STM) at the liquid/solid interface. Synthesized alkoxybenzene derivatives bearing amide group tend to form very large domains of 2-D orderings (>0.25 μm2), whereas the domain size of corresponding urea derivatives was significantly small in the same condition. The quantitative analysis of the concentration dependence of surface coverage using a nucleation-elongation model suggests that the replacement of amide functionality by urea increased the equilibrium constant of the nucleation process of 2-D self-assembly, which is a key factor for the domain size at the liquid/solid interface. Interestingly, the STM observation revealed that a slight difference of molecular structure influences the shape of 2-D ordering domains, and needle-shaped domains with large aspect ratio around 10 were observed by tuning molecule-molecule intramolecular interactions in 2-D self-assembly formed at a liquid/graphite interface." @default.
- W2743139035 created "2017-08-17" @default.
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- W2743139035 date "2017-08-30" @default.
- W2743139035 modified "2023-10-09" @default.
- W2743139035 title "Influence of Multidirectional Interactions on Domain Size and Shape of 2-D Molecular Assemblies" @default.
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- W2743139035 doi "https://doi.org/10.1021/acs.langmuir.7b02094" @default.
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