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• W2743341710 abstract "In this study, CeCu composite catalysts with different Ce/Cu mole ratios were prepared by a hard-template, and their performances in the reverse water–gas shift (RWGS) reaction were investigated. The catalysts were characterized using H2-TPR, XRD, in-situ XPS, AAS, CO2-TPD, and H2-TPD. The characterizations showed that the oxygen vacancies and active Cu0 species as active sites were formed in the CeCu catalysts by the H2 reduction at 400 °C. The synergistic effect of the surface oxygen vacancies and active Cu0 species enhanced catalytic activity of the studied CeCu composite catalysts. The electronic effect between Cu and Ce species boosted the adsorption and activation performances of the reactant CO2 and H2 molecules on the corresponding CeCu catalysts. The Ce1.1Cu1 catalyst demonstrated high stability and the highest CO2 conversion rate in the RWGS reaction, reaching 1.38 mmol gcat−1 min−1 at 400 °C. Its excellent catalytic performance in the RWGS reaction was related to the complete synergistic interaction between the active species via Ce3+-□-Cu0 (□: oxygen vacancy). A CeCu composite material is a superior catalyst for the RWGS reaction because of its high CO2 conversion, 100% CO selectivity, and high stability." @default.
• W2743341710 created "2017-08-17" @default.
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• W2743341710 date "2017-10-01" @default.
• W2743341710 modified "2023-10-15" @default.
• W2743341710 title "CeCu composite catalyst for CO synthesis by reverse water–gas shift reaction: Effect of Ce/Cu mole ratio" @default.
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• W2743341710 doi "https://doi.org/10.1016/j.jcou.2017.07.004" @default.
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