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- W2744208545 abstract "Abstract 2‐Pyrrolines and 6‐oxo‐hexa‐2,4‐dienals have been prepared through the divergent reactions of 1‐benzenesulfonyl‐4‐aryl‐1,2,3‐triazoles with functionalized allenes. The rhodium‐catalyzed reactions between allenols and 1‐benzenesulfonyl‐4‐aryl‐1,2,3‐triazoles yielded 2‐pyrrolines. This transformation is compatible with the presence of aliphatic, aromatic, heterocyclic, amide, and halogen functional groups. Interestingly, a reactivity switch took place when the allene‐tethered alcohol substrate was replaced by its ketone counterpart. When the rhodium‐catalyzed reaction of 1‐benzenesulfonyl‐4‐phenyl‐1,2,3‐triazole was performed with allenones, acyclic 6‐oxo‐hexa‐2,4‐dienals were stereoselectively formed as (2 Z ,4 E ) isomers." @default.
- W2744208545 created "2017-08-17" @default.
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- W2744208545 date "2017-09-04" @default.
- W2744208545 modified "2023-10-15" @default.
- W2744208545 title "Allenols versus Allenones: Rhodium-Catalyzed Regiodivergent and Tunable Allene Reactivity with Triazoles" @default.
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- W2744208545 doi "https://doi.org/10.1002/chem.201702468" @default.
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