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• W2744790240 abstract "The exploration of efficient, stable and cheap water oxidation catalysts (WOCs) is essential for overcoming the bottleneck of water splitting. A series polyoxometalates (POMs) based dinuclear clusters, [M2(β-SiW8O31)2]16− (M = Co2+, Ni2+, Cu2+ and Zn2+) are reported as efficient, robust visible light-driven water oxidation catalysts for the first time. The quite high catalytic turnover number (TON 925), turnover frequency (TOF 7.0 s−1) and 24% quantum yield of [Co2(β-SiW8O31)2]16− (Co-POM) for oxygen evolution are achieved at pH 9.0 using [Ru(bpy)3]2+ as photosensitizer and persulfate as sacrificial electron acceptor. Various experiments including laser flash photolysis, X-ray photoelectron spectra (XPS), UV–vis spectra and IR confirm that Co-POM is the dominant catalyst during water oxidation process. The results offer a utile insight into the design of water oxidation catalysts." @default.
• W2744790240 created "2017-08-17" @default.
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• W2744790240 date "2018-03-01" @default.
• W2744790240 modified "2023-09-27" @default.
• W2744790240 title "Binuclear polyoxometalates based on abundant metals as efficient homogeneous photocatalytic water oxidation catalysts" @default.
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• W2744790240 doi "https://doi.org/10.1016/j.jphotochem.2017.08.016" @default.
• W2744790240 hasPublicationYear "2018" @default.
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