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• W2745805043 startingPage "10257" @default.
• W2745805043 abstract "The scope of direct substitution of the dithiolene ligand from [M(S2C2Ph2)2] [M = Ni2+ (1), Pd2+ (2), Pt2+ (3)] to produce heteroleptic species [M(S2C2Ph2)2Ln] (n = 1, 2) has been broadened to include isonitriles and dithiooxamides in addition to phosphines and diimines. Collective observations regarding ligands that cleanly produce [M(S2C2Ph2)Ln], do not react at all, or lead to ill-defined decomposition identify soft σ donors as the ligand type capable of dithiolene substitution. Substitution of MeNC from [Ni(S2C2Ph2)(CNMe)2] by L provides access to a variety of heteroleptic dithiolene complexes not accessible from 1. Substitution of a dithiolene ligand from 1 involves net redox disproportionation of the ligands from radical monoanions, -S•SC2Ph2, to enedithiolate and dithione, the latter of which is an enhanced leaving group that is subject to further irreversible reactions." @default.
• W2745805043 created "2017-08-31" @default.
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• W2745805043 date "2017-08-18" @default.
• W2745805043 modified "2023-10-16" @default.
• W2745805043 title "Expanding the Scope of Ligand Substitution from [M(S₂C₂Ph₂] (M = Ni²⁺, Pd²⁺, Pt²⁺) To Afford New Heteroleptic Dithiolene Complexes" @default.
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• W2745805043 doi "https://doi.org/10.1021/acs.inorgchem.7b00971" @default.
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• W2745805043 hasPublicationYear "2017" @default.
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