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• W2747622046 endingPage "29659" @default.
• W2747622046 startingPage "29654" @default.
• W2747622046 abstract "Optimization of the interface between the electron transport layer (ETL) and the hybrid perovskite is crucial to achieve high-performance perovskite solar cell (PSC) devices. Fullerene-based compounds have attracted attention as modifiers on the surface properties of TiO2, the archetypal ETL in regular n-i-p PSCs. However, the partial solubility of fullerenes in the aprotic solvents used for perovskite deposition hinders its application to low-temperature solution-processed PSCs. In this work, we introduce a new method for fullerene modification of TiO2 layers derived from nanoparticles (NPs) inks. Atomic force microscopy characterization reveals that the resulting ETL is a network of TiO2-NPs interconnected by fullerenes. Interestingly, this surface modification enhances the bottom interface of the perovskite by improving the charge transfer as well as the top perovskite interface by reducing surface trap states enhancing the contact with the p-type buffer layer. As a result, rigid PSCs reached a 17.2% power conversion efficiency (PCE), while flexible PSCs exhibited a remarkable stabilized PCE of 12.2% demonstrating the potential application of this approach for further scale-up of PSC devices." @default.
• W2747622046 created "2017-08-31" @default.
• W2747622046 creator A5014667154 @default.
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• W2747622046 date "2017-08-24" @default.
• W2747622046 modified "2023-09-26" @default.
• W2747622046 title "Simultaneous Top and Bottom Perovskite Interface Engineering by Fullerene Surface Modification of Titanium Dioxide as Electron Transport Layer" @default.
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• W2747622046 doi "https://doi.org/10.1021/acsami.7b06343" @default.
• W2747622046 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28805366" @default.
• W2747622046 hasPublicationYear "2017" @default.
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