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• W2749695511 abstract "Poly(N-vinyl-2-pyrrolidone) (PVP) of varying molecular weight (M w = 40-360 kDa) were employed to stabilize gold nanoclusters of varying size. The resulting Au:PVP clusters were subsequently used as catalysts for a kinetic study on the sized-dependent aerobic oxidation of 1-indanol, which was monitored by time-resolved in situ infrared spectroscopy. The obtained results suggest that the catalytic behaviour is intimately correlated to the size of the clusters, which in turn depends on the molecular weight of the PVPs. The highest catalytic activity was observed for clusters with a core size of ~7 nm, and the size of the cluster should increase with the molecular weight of the polymer in order to maintain optimal catalytic activity. Studies on the electronic and colloid structure of these clusters revealed that the negative charge density on the cluster surface also strongly depends on the molecular weight of the stabilizing polymers." @default.
• W2749695511 created "2017-08-31" @default.
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• W2749695511 date "2017-08-29" @default.
• W2749695511 modified "2023-10-18" @default.
• W2749695511 title "The Impact of the Polymer Chain Length on the Catalytic Activity of Poly(N-vinyl-2-pyrrolidone)-supported Gold Nanoclusters" @default.
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• W2749695511 doi "https://doi.org/10.1038/s41598-017-10165-9" @default.
• W2749695511 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5575105" @default.
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