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- W2751011014 abstract "Titanium-oxo clusters (TOCs) are important model complexes and potential precise single-source precursors of TiO2 materials. We report here a series of TiO2 samples derived from TOCs with the same wheel-like Ti8O8 clustercore but different stabilizing ligands. Our results demonstrate that the ligands on TOCs not only influence the phase-transition during themolysis, but more importantly tune the photocatalytic H2 evolution activities of the obtained TiO2 materials. Through 500 °C calcination, the nanosized Ti8O8 cluster stabilized by organic benzoate ligands gives rise to a TiO2 sample with H2 production rate of 611 μmol/h/g. When the stabilizing ligands are changed to inorganic SO42−, a significant improvement of H2 evolution activity has been achieved, resulting in a 7-times higher value of 4527 μmol/h/g. This work provides a new strategy to produce TiO2 with enhanced and tunable photocatalytic activities from titanium-oxo cluster precursors." @default.
- W2751011014 created "2017-09-15" @default.
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- W2751011014 date "2017-09-01" @default.
- W2751011014 modified "2023-10-16" @default.
- W2751011014 title "Improving the photocatalytic H2 evolution activities of TiO2 by modulating the stabilizing ligands of the nanoscale Ti8O8-cluster precursors" @default.
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- W2751011014 doi "https://doi.org/10.1016/j.ijhydene.2017.08.083" @default.
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