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• W2751577237 abstract "The gas-phase reactions of [NiL]+ (L=C6 H5 , C5 H4 N, CN) with methane have been explored by using electrospray-ionization mass spectrometry (ESI-MS) complemented by quantum chemical calculations. Though the phenyl Ni complex [Ni(C6 H5 )]+ exclusively abstracts one hydrogen atom from methane at ambient conditions, the cyano Ni complex [Ni(CN)]+ brings about both H-atom abstraction and ligand exchange to generate [Ni(CH3 )]+ . In contrast, the complex 2-pyridinyl Ni [Ni(C5 H4 N)]+ is inert towards this substrate. The presence of the empty 4s(Ni) orbital dominates the proton-coupled electron transfer (PCET) processes for the investigated systems." @default.
• W2751577237 created "2017-09-15" @default.
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• W2751577237 date "2017-09-18" @default.
• W2751577237 modified "2023-10-10" @default.
• W2751577237 title "On the Electronic Origin of Remarkable Ligand Effects on the Reactivities of [NiL]⁺Complexes (L=C₆H₅, C₅H₄N, CN) towards Methane" @default.
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• W2751577237 doi "https://doi.org/10.1002/chem.201703767" @default.
• W2751577237 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28865112" @default.
• W2751577237 hasPublicationYear "2017" @default.
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