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• W2751922829 startingPage "53" @default.
• W2751922829 abstract "DNA footprinting and melting experiments have been used to examine the sequence-specific binding of C8-conjugates of pyrrolobenzodiazepines (PBDs) and benzofused rings including benzothiophene and benzofuran, which are attached using pyrrole- or imidazole-containing linkers. The conjugates modulate the covalent attachment points of the PBDs, so that they bind best to guanines flanked by A/T-rich sequences on either the 5'- or 3'-side. The linker affects the binding, and pyrrole produces larger changes than imidazole. Melting studies with 14-mer oligonucleotide duplexes confirm covalent attachment of the conjugates, which show a different selectivity to anthramycin and reveal that more than one ligand molecule can bind to each duplex." @default.
• W2751922829 created "2017-09-15" @default.
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• W2751922829 date "2017-11-01" @default.
• W2751922829 modified "2023-10-18" @default.
• W2751922829 title "Sequence-selective binding of C8-conjugated pyrrolobenzodiazepines (PBDs) to DNA" @default.
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• W2751922829 doi "https://doi.org/10.1016/j.bpc.2017.08.006" @default.
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