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• W2753146363 abstract "By molecular dynamics simulations coupled with the stochastic polymerization model, we show a certain dependence of the polymer chain polydispersity on the heterogeneity of the initiator sites distribution during surface-initiated polymerization. The heterogeneity of the initiators will lead to change of the mass distribution and the uncontrollability of polydispersity index (PDI) as compared to the homogeneous counterpart. We find a linear master curve of the polymer chain PDI on the interplay of heterogeneity parameter and initiator density, which actually reveals a quantitative dependence of polymer PDI on the free space between neighboring chains. This study helps to better understand and predict the chain polydispersity in the grafted materials via the surface-initiated polymerization." @default.
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• W2753146363 date "2017-08-30" @default.
• W2753146363 modified "2023-10-18" @default.
• W2753146363 title "Dependence of Grafted Polymer Property on the Initiator Site Distribution in Surface-Initiated Polymerization: A Computer Simulation Study" @default.
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• W2753146363 doi "https://doi.org/10.1021/acs.macromol.7b01753" @default.
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