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• W2753664945 abstract "Heusler compounds XY 2 Z with 24 valence electrons per formula unit are potential thermoelectric materials, given their thermal and chemical stability and their relatively earth-abundant constituent elements. We present results on the 24-electron compound TiFe2Sn here. First principles calculations on this compound suggest semiconducting behavior. A relatively flat conduction band that could be associated with a high Seebeck coefficient upon electron doping is found. A series of compounds have been prepared and characterized using a combination of synchrotron x-ray and neutron diffraction studies to understand the effects of site order/disorder phenomena and n-type doping. Samples fabricated by a three step processing approach were subjected to high temperature Seebeck and electrical resistivity measurements. Ti:Fe anti-site disorder is present in the stoichiometric compound and these defects are reduced when starting Ti-rich compositions are employed. Additionally, we investigate control of the Seebeck coefficient through the introduction of carriers through the substitution of Sb on the Sn site in these intrinsically p-type materials." @default.
• W2753664945 created "2017-09-15" @default.
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• W2753664945 date "2017-09-04" @default.
• W2753664945 modified "2023-09-27" @default.
• W2753664945 title "Thermoelectric performance and the role of anti-site disorder in the 24-electron Heusler TiFe₂Sn" @default.
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• W2753664945 doi "https://doi.org/10.1088/1361-648x/aa81e7" @default.
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