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- W2754748548 abstract "Classical nucleation theory is used to consider the solidification of a melt confined between two planar surfaces. The critical nucleus shapes and the associated nucleation energy barriers are computed as a function of the thickness of the film and the film's relevant bulk and interface energies. The analysis is then repeated for the melting transition, and expressions for the depression and elevation of the melting temperature, relative to the thermodynamic bulk melting temperature of the film material, are found. A nucleus morphology diagram is constructed. This diagram presents the lowest energy morphology of the nuclei, as well as melting points, as a function of the system parameters. Using the nucleus morphology diagram, experimental and system parameters that allow for the desired nucleation behavior can be identified. Furthermore, the nucleus morphology diagram illustrates a region of parameter space where the film is predicted to solidify above its thermodynamic bulk melting temperature, a behavior termed presolidification. The theory is used to predict the temperature at which the nucleation of the solid phase and liquid phase is expected for Ge between two glass substrates. Furthermore, a possible route for controlling the orientation of the film is identified. By controlling the growth temperature, certain orientations may not be able to nucleate, thereby reducing the possible number of orientations within a film." @default.
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- W2754748548 date "2017-09-14" @default.
- W2754748548 modified "2023-09-27" @default.
- W2754748548 title "Nucleation of melting and solidification in confined high aspect ratio thin films" @default.
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- W2754748548 doi "https://doi.org/10.1063/1.4997583" @default.
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