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• W2756451010 abstract "Tailoring the morphology and microstructure of electrocatalysts is important in improving catalytic performance. Herein, porous multishelled Ni2P hollow microspheres assembled by nanoparticles were prepared through a simple and economical self-templating approach followed by phosphorization. Compared with nanoparticles and hierarchical solid-interior microspheres, the synthesized multishelled, hollow microstructures of Ni2P exhibit significantly higher electrocatalytic activity for the hydrogen evolution reaction in a 1 M KOH electrolyte. Additionally, a NiOOH layer is formed on the surface of Ni2P during anodic polarization, as revealed by electron microscopy, X-ray photoelectron spectroscopy, and in situ Raman analysis. The Ni2P/NiOOH derivative outperforms the benchmark RuO2 in catalyzing the oxygen evolution reaction. Furthermore, pairing the carbon fiber paper-supported multishelled Ni2P as both the anode and cathode results in superior overall alkaline water splitting performance, generating 10 and ..." @default.
• W2756451010 created "2017-09-25" @default.
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• W2756451010 date "2017-10-02" @default.
• W2756451010 modified "2023-10-16" @default.
• W2756451010 title "Porous Multishelled Ni₂P Hollow Microspheres as an Active Electrocatalyst for Hydrogen and Oxygen Evolution" @default.
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• W2756451010 doi "https://doi.org/10.1021/acs.chemmater.7b03627" @default.
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