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• W2759301061 abstract "The reduction of charge carrier recombination and intrinsic defect density in organic–inorganic halide perovskite absorber materials is a prerequisite to achieving high-performance perovskite solar cells with good efficiency and stability. Here, we fabricated inverted planar perovskite solar cells by incorporation of a small amount of excess organic/inorganic halide (methylammonium iodide (CH3NH3I; MAI), formamidinium iodide (CH(NH2)2I; FAI), and cesium iodide (CsI)) in CH3NH3PbI3 perovskite film. Larger crystalline grains and enhanced crystallinity in CH3NH3PbI3 perovskite films with excess organic/inorganic halide reduce the charge carrier recombination and defect density, leading to enhanced device efficiency (MAI+: 14.49 ± 0.30%, FAI+: 16.22 ± 0.38% and CsI+: 17.52 ± 0.56%) compared to the efficiency of a control MAPbI3 device (MAI: 12.63 ± 0.64%) and device stability. Especially, the incorporation of a small amount of excess CsI in MAPbI3 perovskite film leads to a highly reproducible fill factor of over 83%, increased open-circuit voltage (from 0.946 to 1.042 V), and short-circuit current density (from 18.43 to 20.89 mA/cm2)." @default.
• W2759301061 created "2017-10-06" @default.
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• W2759301061 date "2017-10-04" @default.
• W2759301061 modified "2023-10-15" @default.
• W2759301061 title "High-Performance CH₃NH₃PbI₃-Inverted Planar Perovskite Solar Cells with Fill Factor Over 83% via Excess Organic/Inorganic Halide" @default.
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• W2759301061 doi "https://doi.org/10.1021/acsami.7b11083" @default.
• W2759301061 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28948770" @default.
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