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• W2760879870 abstract "The authors report on recrystallization of VO2 films on Al2O3 (001) single crystalline substrates into (011)-oriented large grains. In the VO2 films deposited by biased reactive sputtering, (011)-oriented micrometer-sized grains were found to coexist with commonly observed (010)-oriented nanometer-sized grains. Characteristic maps of oxygen concentrations observed using an electron probe microanalyzer for areas with and without (011)-oriented grains suggest recrystallization phenomena of (020)-oriented grains in the existence of VOx (x > 2) phases, where the growth mode in the Thornton model is able to enter the recrystallization zone in which the ratio of substrate temperature (Ts) to melting temperature (Tm) exceeds 0.7. Accordingly, rapid grain boundary migrations and bulk diffusions would occur during sputtering deposition and result in the occurrence of the recrystallization phenomena. Recrystallized (011)-oriented micrometer-sized grains underwent structural phase transition (SPT) through the intermediate M2 phase, suggesting a significant role of crystalline orientation and size, in addition to the elongation of the V–V distance along the cR-axis. Micro-Raman mapping showed that (011)-oriented grains possess characteristic features in crystallinity compared to (020)-oriented grains, giving the possibility for controlling SPT of VO2 on Al2O3 (001) in the present study." @default.
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• W2760879870 date "2017-11-01" @default.
• W2760879870 modified "2023-09-27" @default.
• W2760879870 title "Recrystallization of VO2 films into (011)-oriented micrometer-sized grains on Al2O3 (001) in biased reactive sputtering" @default.
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• W2760879870 doi "https://doi.org/10.1116/1.4989669" @default.
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