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• W2762819762 abstract "We propose a novel approach to cavity-ring-down-spectroscopy (CRDS) in which spectra acquired with a frequency-agile rapid-scanning (FARS) scheme, i.e., with a laser sideband stepped across the modes of a high-finesse cavity, are interleaved with one another by a sub-millisecond readjustment of the cavity length. This brings to time acquisitions below 20 s for few-GHz-wide spectra composed of a very high number of spectral points, typically 3200. Thanks to the signal-to-noise ratio easily in excess of 10 000, each FARS-CRDS spectrum is shown to be sufficient to determine the line-centre frequency of a Doppler broadened line with a precision of 2 parts over 1011, thus very close to that of sub-Doppler regimes and in a few-seconds time scale. The referencing of the probe laser to a frequency comb provides absolute accuracy and long-term reproducibility to the spectrometer and makes it a powerful tool for precision spectroscopy and line-shape analysis. The experimental approach is discussed in detail together with experimental precision and accuracy tests on the (30 012) ← (00 001) P12e line of CO2 at ∼1.57 μm." @default.
• W2762819762 created "2017-10-20" @default.
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• W2762819762 date "2017-10-05" @default.
• W2762819762 modified "2023-10-17" @default.
• W2762819762 title "Conjugating precision and acquisition time in a Doppler broadening regime by interleaved frequency-agile rapid-scanning cavity ring-down spectroscopy" @default.
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• W2762819762 doi "https://doi.org/10.1063/1.4999056" @default.
• W2762819762 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28987101" @default.
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