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- W2765096975 abstract "Herein, we developed an efficient and selective nickel-catalyzed monoalkylation of various primary alcohols with aryl and heteroaryl amines together with diols and amino alcohol derivatives. Notably, the catalytic protocol consisting of an earth-abundant and non-precious NiBr2/L1 system enables the transformations in the presence of hydroxyl, alkene, nitrile, and nitro functionalities. As a highlight, we have demonstrated the alkylation of diamine, intramolecular cyclization to N-heterocycles, and functionalization of complex vitamin E, an (±)-α-tocopherol derivative. Preliminary mechanistic studies revealed the participation of a benzylic C–H bond in the rate-determining step." @default.
- W2765096975 created "2017-11-10" @default.
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- W2765096975 creator A5021823749 @default.
- W2765096975 creator A5058836983 @default.
- W2765096975 date "2017-10-31" @default.
- W2765096975 modified "2023-10-03" @default.
- W2765096975 title "An Efficient and Selective Nickel-Catalyzed Direct N-Alkylation of Anilines with Alcohols" @default.
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- W2765096975 doi "https://doi.org/10.1021/acscatal.7b02817" @default.
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