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- W2765223353 abstract "Adsorption of CO2 under humid conditions is important, as flue gases contain some degree of moisture, while aqueous-phase sensing of nitro-aromatic compounds is critical for environmental protection and anti-terrorism activities. However, implementing both of these aspects in metal–organic frameworks (MOFs) is rare and challenging due to their moisture instability. To this end, we prepared three isostructural, pillar-layer Zn(II) MOFs where criss-cross pillaring by the linkers tunes the pore opening and pore electronic environment that in turn modulate thermal and/or moisture stabilities. While activated 2 (2′), incorporating an azo group in the linker, exhibits excellent CO2/N2 selectivity (>200), 1′, containing a 4,4′-bipyridine linker displays superior hydrolytic stability with minimum loss in CO2 adsorption–desorption cycles up to 10 days of water vapor exposure. However, framework 3, with a bis(4-pyridyl)ethylene linker, is unstable. Importantly, aqueous-phase sensitive detection of picric acid (PA) ..." @default.
- W2765223353 created "2017-11-10" @default.
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- W2765223353 date "2017-11-01" @default.
- W2765223353 modified "2023-09-26" @default.
- W2765223353 title "Construction of Pillar-Layer Metal–Organic Frameworks for CO<sub>2</sub> Adsorption under Humid Climate: High Selectivity and Sensitive Detection of Picric Acid in Water" @default.
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- W2765223353 doi "https://doi.org/10.1021/acssuschemeng.7b02087" @default.
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