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- W2765258731 abstract "Nd was used as the modifier to improve the NH3-selective catalytic reduction (SCR) performance of MnOx catalyst used in NOx abatement. The results of the activity test indicated that MnNdOx-0.1 catalyst displayed remarkable catalytic activity and N2 selectivity in the temperature range of 50–300 °C. Characterization results proved the enhanced reducibility and the facilitated NH3 and NOx adsorption over MnNdOx-0.1 catalyst, accompanied by the existence of more Mn4+ and surface adsorbed oxygen species over its surface. The results of the in situ diffuse reflectance infrared Fourier transform study pointed out that the NH3-SCR reaction over the MnNdOx-0.1 catalyst was mainly under the control of the Langmuir–Hinshelwood mechanism (≤100 °C); when the reaction temperature was over 200 °C, the Eley–Rideal mechanism was dominant. More adsorbed NOx and NH3 species over the MnNdOx-0.1 catalyst, along with the activation effect of Nd on the adsorbed reactants, had a facilitation impact on the SCR reaction process over the MnNdOx-0.1 catalyst." @default.
- W2765258731 created "2017-11-10" @default.
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- W2765258731 date "2017-10-31" @default.
- W2765258731 modified "2023-09-26" @default.
- W2765258731 title "A Highly Effective MnNdOx Catalyst for the Selective Catalytic Reduction of NO<i><sub>x</sub></i> with NH<sub>3</sub>" @default.
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- W2765258731 doi "https://doi.org/10.1021/acs.iecr.7b03705" @default.
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