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- W2765296976 abstract "We investigated CuWO4 as a promising photoanode and its surface functionalization with Ag2NCN. The composite photoanode displays a synergetic effect between its constituents during photoelectrochemical (PEC) water oxidation. After placing Ag2NCN particles on the CuWO4 thin film, the photocurrent density increases from 15 to 45 μA cm–2 at 1.23 V vs reversible hydrogen electrode (RHE) in phosphate buffer electrolyte at pH 7 under simulated AM1.5 G illumination. The different positions of the band edges of CuWO4 and Ag2NCN favor charge carrier separation at their interface. Upon illumination, photogenerated electrons of both semiconductors are transferred to the conduction band and can migrate to the counterelectrode. The higher position of the conduction band edge of Ag2NCN allows its electrons to be injected into the conduction band of CuWO4. Simultaneously, holes from the cyanamide are blocked, because the valence band edge position of CuWO4 is positioned lower than for Ag2NCN. This results in more effici..." @default.
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- W2765296976 date "2017-11-20" @default.
- W2765296976 modified "2023-09-24" @default.
- W2765296976 title "Enhanced Photoelectrochemical Water Oxidation Efficiency of CuWO<sub>4</sub> Photoanodes by Surface Modification with Ag<sub>2</sub>NCN" @default.
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- W2765296976 doi "https://doi.org/10.1021/acs.jpcc.7b10220" @default.
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