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• W2765332893 abstract "Recently, $mathrm{Pb}(mathrm{I}{mathrm{n}}_{1/2}mathrm{N}{mathrm{b}}_{1/2}){mathrm{O}}_{3}text{ensuremath{-}}mathrm{PbZr}{mathrm{O}}_{3}text{ensuremath{-}}mathrm{Pb}(mathrm{M}{mathrm{g}}_{1/3}mathrm{N}{mathrm{b}}_{2/3}){mathrm{O}}_{3}text{ensuremath{-}}mathrm{PbTi}{mathrm{O}}_{3}$ (PIN-PZ-PMN-PT) relaxor single crystals were demonstrated to possess improved temperature-insensitive properties, which would be desirable for high-power device applications. The relaxor character associated with the development of local random fields (RFs) and a high rhombohedral-tetragonal (R-T) ferroelectric transition temperature $({T}_{mathrm{R}ensuremath{-}mathrm{T}}>120{phantom{rule{0.16em}{0ex}}}^{ensuremath{circ}}mathrm{C})$ would be critical for the excellent properties. A significant effect of the chemical substitution of $mathrm{I}{mathrm{n}}^{3+}$ and $mathrm{Z}{mathrm{r}}^{4+}$ in PMN-PT to give PIN-PZ-PMN-PT is the development of local strain heterogeneity, which acts to suppress the development of macroscopic shear strains without suppressing the development of local ferroelectric moments and contribute substantially to the RFs in PIN-PZ-PMN-PT. Measurements of elastic and anelastic properties by resonant ultrasound spectroscopy show that PIN-PZ-PMN-PT crystal has a quite different form of elastic anomaly due to Vogel-Fulcher freezing, rather than the a discrete cubic-$T$ transition seen in a single crystal of PMN-28PT. It also has high acoustic loss of the relaxor phase down to ${T}_{mathrm{R}ensuremath{-}mathrm{T}}$. Analysis of piezoresponse force microscopy phase images at different temperatures provides a quantitative insight into the extent to which the RFs influence the microdomain structure and the short-range order correlation length $ensuremath{langle}ensuremath{xi}ensuremath{rangle}$." @default.
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• W2765332893 date "2017-10-18" @default.
• W2765332893 modified "2023-10-14" @default.
• W2765332893 title "Local strain heterogeneity and elastic relaxation dynamics associated with relaxor behavior in the single-crystal perovskite <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mi>Pb</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mrow><mml:mi mathvariant=normal>I</mml:mi><mml:msub><mml:mi mathvariant=normal>n</mml:mi><mml:mrow><mml:mn>1</mml:mn><mml:mo>/</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msub><mml:mi mathvariant=normal>N</mml:mi><mml:msub><mml:mi mathvariant=normal…" @default.
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• W2765332893 doi "https://doi.org/10.1103/physrevb.96.144109" @default.
• W2765332893 hasPublicationYear "2017" @default.
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