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- W2765385938 abstract "We calculate the oxygen $K$-edge x-ray magnetic circular dichroism (XMCD) spectra of ${mathrm{CrO}}_{2}$ to investigate the origin of light-element XMCD. The XMCD spectra evaluated by using a multiple scattering theory are interpreted in terms of the spin-orbit interaction (SOI) at each atomic site. We find that the SOI at the nearest-neighbor Cr atoms dominantly contributes to the oxygen $K$-edge XMCD. Since it has been speculated that XMCD originates from the spin polarization and the SOI at the x-ray-absorbing atom, the present finding may lead to modification of the previously speculated mechanism underlying $K$-edge XMCD. We also perform calculations with a small ${mathrm{CrO}}_{2}$ cluster to examine how the O-$p$ and Cr-$d$ states are hybridized and how oxygen atoms acquire orbital angular momentum density. Strong $K$-edge XMCD features reflect the character of the $d$ states of neighboring magnetic atoms and do not directly connect to the orbital magnetic moments of light-element $p$ states." @default.
- W2765385938 created "2017-11-10" @default.
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- W2765385938 date "2017-10-17" @default.
- W2765385938 modified "2023-10-12" @default.
- W2765385938 title "Effects of spin-orbit interaction in chromium on oxygen K -edge x-ray magnetic circular dichroism spectra in CrO2" @default.
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- W2765385938 doi "https://doi.org/10.1103/physrevb.96.144419" @default.
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