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- W2765829173 abstract "The effect of irreversibly adsorbed Bi on commercial Pt/C catalyst toward glucose electro-oxidation reaction (GOR) in different electrolytes (acidic, neutral, alkaline) is studied. Bi is successfully deposited on Pt/C from Bi3+ containing acidic solution from 0 to 90% coverage degree. The stability of the Bi layer in acid and alkaline corresponded to previous studies and started to dissolve at 0.7 V and 0.8 V versus reversible hydrogen electrode (RHE), respectively. However, in neutral phosphate buffer the layer showed remarkable stability to at least 1.2 V versus RHE. Bi modification at low (20%) and high (80%) coverage showed the highest increase in the activity of Pt/C toward GOR by a factor up to 7 due to the increased poisoning resistance of the modified catalyst. The effect of poisoning was especially reduced at high Bi coverage (80%), which shows that adsorbate blocked by Bi through the third-body effect is effective. Finally, with or without Bi modification GOR on Pt/C was most active in alkaline conditions." @default.
- W2765829173 created "2017-11-10" @default.
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- W2765829173 date "2018-09-01" @default.
- W2765829173 modified "2023-10-03" @default.
- W2765829173 title "Activation of commercial Pt/C catalyst toward glucose electro-oxidation by irreversible Bi adsorption" @default.
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- W2765829173 doi "https://doi.org/10.1016/j.jechem.2017.09.030" @default.
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