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• W2766147810 abstract "The first examples of kinetically controlled cross-metathesis reactions that generate Z- or E-trisubstituted alkenes are disclosed. Transformations are catalyzed by ≤6.0 mol % of a Ru catechothiolate complex and afford trisubstituted allylic alcohols and ethers in up to 81% yield and >98% stereoisomeric purity. The method has considerable scope, as olefins containing an alcohol, an aldehyde, an epoxide, a carboxylic acid, or an alkenyl group may be used. Mechanistic models that account for the observed levels and trends in efficiency and stereochemical control are provided, based on DFT studies." @default.
• W2766147810 created "2017-11-10" @default.
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• W2766147810 date "2017-10-25" @default.
• W2766147810 modified "2023-10-09" @default.
• W2766147810 title "Synthesis of <i>Z</i>- or <i>E</i>-Trisubstituted Allylic Alcohols and Ethers by Kinetically Controlled Cross-Metathesis with a Ru Catechothiolate Complex" @default.
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• W2766147810 doi "https://doi.org/10.1021/jacs.7b10010" @default.
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