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- W2766341738 abstract "A method for the organocatalytic, highly enantioselective, and moderately diastereoselective dimerization (redox isomerization/acetal formation) of γ‐hydroxyenones is disclosed. The stereogenic acetal products were obtained via hemiacetal intermediates followed by a cyclization reaction. With bifunctional thiourea catalysts, high yields and excellent enantioselectivities were achieved for a variety of acetal products under mild reaction conditions. In addition, detailed DFT calculations were performed to investigate the mechanism of this reaction, and these calculations suggested that the diastereoselectivity was due to a kinetically controlled process." @default.
- W2766341738 created "2017-11-10" @default.
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- W2766341738 date "2017-12-19" @default.
- W2766341738 modified "2023-09-25" @default.
- W2766341738 title "Organocatalytic Asymmetric Dimerization of γ-Hydroxyenones to Acetals and Theoretical Investigations into the Diastereoselection" @default.
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- W2766341738 doi "https://doi.org/10.1002/ejoc.201701439" @default.
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