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- W2766394023 abstract "Abstract A series of multifunctional nanoporous organic polymers with high microporosity have been successfully synthesized via Friedel-Crafts alkylation and Scholl coupling reactions. Porous properties are well-controllable by simply regulating the lengths and rigidities of linkers, where the rigid tetrahedral building block, i.e. 1,3,5,7-tetraphenyladamantane, knitted with flexible alkyl chains leads to a hierarchically porous structure of NOP-53. Such amorphous materials derived from the high rigid building block achieve high surface areas (1178 m2 g−1 for NOP-54) and substantially improved micro-pore volumes (0.86 cm3 g−1, Vmicro/Vtotal = 65%). The as-made porous network NOP-54 featuring highest microporosity can uptake 14.2 wt% CO2 at 273 K and 1 bar, and good selectivity ratios for CO2 adsorption over N2 (56.1) and CH4 (13.9) at 273 K are achieved. Furthermore, such polymers display excellent iodine vapor uptake of up to 202 wt% and shows remarkable capability as iodine sorbent in solution. These results are significant for constructing accessible aromatic networks with promoted microporosity targeting for environmental challenges." @default.
- W2766394023 created "2017-11-10" @default.
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- W2766394023 date "2018-02-01" @default.
- W2766394023 modified "2023-10-17" @default.
- W2766394023 title "Versatile Adamantane-based porous polymers with enhanced microporosity for efficient CO2 capture and iodine removal" @default.
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- W2766394023 doi "https://doi.org/10.1016/j.cej.2017.10.133" @default.
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