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• W2766528074 abstract "Abstract The multifaceted character of 5 f electrons in actinide materials, from localized to itinerant and in between, together with their complex interactions with 6 d and other conduction electron states, has thwarted efforts for fully understanding this class of compounds. While theoretical efforts abound, direct experimental probes of relevant electronic states and their hybridization are limited. Here we exploit the presence of sizable quadrupolar and dipolar contributions in the uranium L 3 -edge X-ray absorption cross section to provide unique information on the extent of spin-polarized hybridization between 5 f and 6 d electronic states by means of X-ray magnetic circular dichroism. As a result, we show how this 5 f -6 d hybridization regulates the magnetism of each sublattice in UCu 2 Si 2 and UMn 2 Si 2 compounds, demonstrating the potentiality of this methodology to investigate a plethora of magnetic actinide compounds." @default.
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• W2766528074 date "2017-10-31" @default.
• W2766528074 modified "2023-10-10" @default.
• W2766528074 title "Unraveling 5f-6d hybridization in uranium compounds via spin-resolved L-edge spectroscopy" @default.
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• W2766528074 doi "https://doi.org/10.1038/s41467-017-01524-1" @default.
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