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- W2767332364 abstract "The constitutive modelling of semi-crystalline polymers seeks to obtain reliable predictive tools for a wide range of their mechanical responses. Such efforts have continued to occupy computational material scientists. Although significant advances have been made regarding amorphous polymers, thanks to works by Buckley [1], Boyce [2], and Govaert [3], there is significant research scope for developing similar predictive modelling fidelity for semi-crystalline polymers. The presence of crystalline and amorphous phases in semi-crystalline polymers presents interesting constitutive modelling challenges.In this study, a physically based, three-dimensional constitutive model has been developed for simulating a wide range of features observed in deformation and processing of semi-crystalline polymers. The constitutive mathematics is based on a one-process Grass-Rubber model for amorphous polymers proposed by Buckley and colleagues [1]. The model philosophy exploits the presence of multiple relaxation processes associated with the different mechanics of the crystalline, amorphous and pseudo-amorphous parts of the polymer. The model development reasoning is inspired by a well-known physical framework of rate-dependent deformation that establishes a correlation between the observed transition in flow stress of a material and the secondary β-transition of the viscoelastic behaviour. Here, two dominant relaxation processes were identified - the α- and the β-processes. Each process was modelled using the bond-stretching and conformational stresses constitutive mathematics of the Glass-Rubber model.The model has been implemented numerically into a commercial finite element code through a user-defined material subroutine (UMAT) and validated against compression test results carried out on an isotactic polypropylene across an unusually wide range of strain rates [4]. In this study, the model predicts quite well the experimentally observed nonlinear mechanical responses like: temperature and rate-dependence, adiabatic heating effects, structural rejuvenation and post-yield de-ageing of polypropylene. It provides a viable modelling tool that can be utilized for design involving semicrystalline polymers at room temperature as well as exploring the processing response at elevated temperatures." @default.
- W2767332364 created "2017-11-17" @default.
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- W2767332364 date "2017-09-07" @default.
- W2767332364 modified "2023-09-27" @default.
- W2767332364 title "A constitutive model for semi-crystalline polymers: A multiple viscoelastic relaxation processes implementation." @default.
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