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- W2767631944 abstract "Highly regiodivergent copper-catalyzed allylic/propargylic difluoromethylation reactions by employing different ligands are described. When 5,6-dimethyl-1,10-phenanthroline was used as the ligand, exclusively α-difluoromethylated products were obtained, while γ-selective difluoromethylated products were generated when N-heterocyclic carbene-SIPr was used as the ligand. Likewise, high α- vs. γ-selectivities were achieved in the presence of similar copper catalysts for the reactions of propargyl bromides. Moreover, a copper-catalyzed asymmetric allylic difluoromethylation reaction with moderate to good enantioselectivity by the use of chiral ligands was developed." @default.
- W2767631944 created "2017-11-17" @default.
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- W2767631944 date "2017-11-27" @default.
- W2767631944 modified "2023-10-01" @default.
- W2767631944 title "Ligand-Controlled Copper-Catalyzed Highly Regioselective Difluoromethylation of Allylic Chlorides/Bromides and Propargyl Bromides" @default.
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- W2767631944 doi "https://doi.org/10.1002/cjoc.201700594" @default.
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