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- W2767713088 endingPage "1701953" @default.
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- W2767713088 abstract "The use of selenium as a cathode in rechargeable sodium–selenium batteries is hampered by low Se loading, inferior electrode kinetics, and polyselenide shuttling between the cathode and anode. Here a high-performance sodium–selenium cell is presented by coupling a binder-free, self-interwoven carbon nanofiber–selenium cathode with a light-weight carbon-coated bifunctional separator. With this strategy, electrodes with a high Se mass loading (4.4 mg cm−2) render high reversible capacities of 599 mA h g−1 at 0.1C rate and 382 mA h g−1 at 5C rate. In addition, this novel cell offers good shelf-life with a low self-discharge, retaining 93.4% of its initial capacity even after resting for six months. As evidenced by experimental and density functional theory analysis, the remarkable dynamic (cycle life) and static (shelf-life) stabilities originate from the high electrical conductivity, improved Na-ion accessibility through the 3D interconnected open channels, and highly restrained polyselenide shuttle. The results demonstrate the viability of high-performance sodium–selenium batteries with high selenium loading." @default.
- W2767713088 created "2017-11-17" @default.
- W2767713088 creator A5028316310 @default.
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- W2767713088 date "2017-11-08" @default.
- W2767713088 modified "2023-10-10" @default.
- W2767713088 title "Long Cycle Life, Low Self‐Discharge Sodium–Selenium Batteries with High Selenium Loading and Suppressed Polyselenide Shuttling" @default.
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- W2767713088 doi "https://doi.org/10.1002/aenm.201701953" @default.
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