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• W2768014789 endingPage "1158" @default.
• W2768014789 startingPage "1150" @default.
• W2768014789 abstract "Different configurations of Sn and C films were deposited and used as a planar anode for Li ion battery. The interplay of carbon layer with Sn as supporting and buffering, respectively, was revealed. The suppression on the allotropic transformation to α phase by a carbon layer results in a significantly improved capacity retention rate, which also avoids the crack of Sn film. As expected, a conductive carbon layer improves rating performance. However, a supporting carbon layer (SC) just contributes to the charge transfer process. A DFT approach was used to assess the allotropic transformation process. An additional barrier (∼0.86 eV) exits on the α-β diagram, which is responsible for the irreversibility of α phase back to β phase. An enhanced persistence of β phase in Sn/C anode contributes to cycling performance. A Li rich condition contributes to the stabilization of β-Sn, which is thermodynamically favored. A nano buffering carbon (BC) layer can evidently alleviate the side reaction on Sn surface, which in turn promotes the diffusion of Li ions in electrode and generates a Li rich condition. The direct contact of Sn with electrolyte leads to serious accumulation of α-Sn during cycling and results in a poor cycling performance. By the synergistic effect of BC and SC, a sandwich C/Sn/C structure demonstrates an enchantment in electrochemical behavior." @default.
• W2768014789 created "2017-11-17" @default.
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• W2768014789 date "2018-03-01" @default.
• W2768014789 modified "2023-10-16" @default.
• W2768014789 title "Suppression on allotropic transformation of Sn planar anode with enhanced electrochemical performance" @default.
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• W2768014789 doi "https://doi.org/10.1016/j.apsusc.2017.11.079" @default.
• W2768014789 hasPublicationYear "2018" @default.
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