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- W2768024814 abstract "Photochemical precursors that produce dA• and dG(N2–H)• are needed to investigate their reactivity. The synthesis of two 1,1-diphenylhydrazines (1, 2) and their use as photochemical sources of dA• and dG(N2–H)• is presented. Trapping studies indicate production of these radicals with good fidelity, and 1 was incorporated into an oligonucleotide via solid-phase synthesis. Cyclic voltammetric studies show that reduction potentials of 1 and 2 are lower than those of widely used “hole sinks”, e.g., 8-oxodGuo and 7-deazadGuo, to investigate DNA–hole transfer processes. These molecules could be useful (a) as sources of dA• and dG(N2–H)• at specific sites in oligonucleotides and (b) as “hole sinks” for the study of DNA–hole transfer processes." @default.
- W2768024814 created "2017-11-17" @default.
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- W2768024814 date "2017-11-10" @default.
- W2768024814 modified "2023-09-22" @default.
- W2768024814 title "Independent Photochemical Generation and Reactivity of Nitrogen-Centered Purine Nucleoside Radicals from Hydrazines" @default.
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- W2768024814 doi "https://doi.org/10.1021/acs.orglett.7b03368" @default.
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