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- W2768045262 abstract "A highly efficient and stereoselective route to potential synthetic intermediates for ocellenyne and related C15 acetogenin natural products with 6,10-syn- and 6,10-anti-2,5-dioxabicyclo[2.2.1]heptane core structures has been developed by means of an iterative biogenesis-inspired oxonium ion formation/fragmentation sequence. In accordance with chemical transformations, the most likely stereostructure for (E)-ocellenyne on the basis of GIAO 13C NMR calculations possesses a 6,10-anti-2,5-dioxabicyclo[2.2.1]heptane core, as predicted from a plausible biosynthetic pathway, instead of the spectroscopically proposed 6,10-syn-2,5-dioxabicyclo[2.2.1]heptane skeleton." @default.
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- W2768045262 date "2017-11-07" @default.
- W2768045262 modified "2023-10-16" @default.
- W2768045262 title "Construction of 6,10-<i>syn</i>- and -<i>anti</i>-2,5-Dioxabicyclo[2.2.1]heptane Skeletons via Oxonium Ion Formation/Fragmentation: Prediction of Structure of (<i>E</i>)-Ocellenyne by NMR Calculation" @default.
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- W2768045262 doi "https://doi.org/10.1021/acs.orglett.7b03226" @default.
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