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- W2768099069 abstract "We describe Stark-induced adiabatic Raman passage (SARP), a technique that we have extensively developed in our laboratory to prepare vibrationally excited single and superposition of quantum states of molecules with a large population density in a collision-free ambience, such as in a molecular beam. We present a theoretical framework of SARP using Schrödinger and density matrix equations. A Bloch-Feynman vector model picture is constructed to provide an intuitive and pictorial description of the Stark-induced adiabatic population transfer. Experimental results are presented in support of our theoretical simulations of SARP preparing both single and superpositions of rovibrational M-quantum states with near-complete population transfer. Additionally, we introduce a new Stark-induced adiabatic ladder climbing technique that is able to selectively populate a high-lying vibrational quantum state near dissociation. Brief descriptions of other related adiabatic passage processes, such as stimulated Raman adiabatic passage (STIRAP) and Stark-chirped rapid adiabatic passage (SCRAP), are added for completeness and for comparison with SARP." @default.
- W2768099069 created "2017-12-04" @default.
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- W2768099069 date "2018-01-01" @default.
- W2768099069 modified "2023-10-16" @default.
- W2768099069 title "Stark-Induced Adiabatic Passage Processes to Selectively Prepare Vibrationally Excited Single and Superposition of Quantum States" @default.
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- W2768099069 doi "https://doi.org/10.1016/b978-0-12-811220-5.00001-0" @default.
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