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- W2768492054 abstract "Nanocsrystals of Zn(pyrz)2(SiF6) (or SIFSIX-3-Zn) metal-organic framework were synthesized by a facile sonochemical means and incorporated into a polyimide membrane to realize an excellent CO2/CH4 separation performance. Zn(pyrz)2(SiF6) nanocrystals selectively took up a large amount of CO2 even at low pressure while negligible uptake was observed for CH4. This implies that Zn(pyrz)2(SiF6) is an ideal filler to improve CO2/CH4 separation performance of polymer membrane via selective transport of CO2 over CH4. Subsequently, high-quality mixed-matrix membranes that are free of filler/polymer interfacial voids were successfully fabricated by employing house-made polyimide as a polymer matrix. Binary CO2/CH4 mixture gas permeation tests revealed that both CO2 permeability and CO2/CH4 selectivity of mixed-matrix membranes, especially for the membrane with 20 wt% filler loading, were significantly improved compared to those of pure polymeric membrane owing to the selective CO2 uptake and transport by Zn(pyrz)2(SiF6) crystals. As a result, a high performance surpassing the upper bound limit for polymeric membranes was achieved." @default.
- W2768492054 created "2017-12-04" @default.
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- W2768492054 date "2018-04-01" @default.
- W2768492054 modified "2023-10-16" @default.
- W2768492054 title "High performance composite membranes comprising Zn(pyrz) 2 (SiF 6 ) nanocrystals for CO 2 /CH 4 separation" @default.
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- W2768492054 doi "https://doi.org/10.1016/j.jiec.2017.11.014" @default.
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