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• W2768663505 startingPage "475" @default.
• W2768663505 abstract "A novel Au36-xCux(m-MBT)24 (x = 1-3, m-MBT = 3-methylbenzenethiolate) nanocluster has been prepared. According to the X-ray single crystal diffractometer, the structure of Au36-xCux(m-MBT)24 is similar to that of Au36(SPhtBu)24. The Au36-xCux(m-MBT)24 nanocluster contains a face-centered cubic (FCC) M28 core, which is protected by 4 M2S3 (M = Au/Cu) staple motifs and 12 bridging SR ligands. The Cu dopants could possibly occupy 14 sites (six in the sub-surface and eight in the staple motifs). Spectral monitoring indicates that the number of Cu dopants sequentially increased on increasing the amount of Cu precursors (relative to a Au control). Meanwhile, DFT calculations imply that the maximum doping number of Cu is 3, and doping occurs preferentially at the staple sites and sub-surface sites (instead of the centre of the core). Because the atomic orbital of the peripheral locations hardly contributes to the frontier molecular orbitals, the UV-vis of the AuCu alloy is almost the same as that of its homometallic Au counterpart." @default.
• W2768663505 created "2017-12-04" @default.
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• W2768663505 date "2018-01-01" @default.
• W2768663505 modified "2023-10-14" @default.
• W2768663505 title "X-ray crystal structure and doping mechanism of bimetallic nanocluster Au_36−xCu_x(<i>m</i>-MBT)₂₄(<i>x</i>= 1–3)" @default.
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• W2768663505 doi "https://doi.org/10.1039/c7dt02959d" @default.
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• W2768663505 hasPublicationYear "2018" @default.
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