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- W2769535519 abstract "1H–71Ga internuclear spatial proximity/interaction between Brønsted acid site (BAS) and cationic Ga species (Lewis acid sites) in Ga-modified ZSM-5 zeolites, which leads to a synergic effect in the methanol-to-aromatics (MTA) conversion, was identified with solid-state NMR spectroscopy. The internuclear distance between BAS and Ga species was measured, which is similar to that of a neighboring BAS pair located in the six-membered rings of ZSM-5. The Brønsted acidity of the Ga-modified zeolite was considerably enhanced due to the synergic effect, and the synergic active sites were quantified by 1H–71Ga double-resonance solid-state NMR, which shows a correlation with the aromatics selectivity in the MTA reaction." @default.
- W2769535519 created "2017-12-04" @default.
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- W2769535519 date "2017-11-28" @default.
- W2769535519 modified "2023-10-14" @default.
- W2769535519 title "Brønsted/Lewis Acid Synergy in Methanol-to-Aromatics Conversion on Ga-Modified ZSM-5 Zeolites, As Studied by Solid-State NMR Spectroscopy" @default.
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- W2769535519 doi "https://doi.org/10.1021/acscatal.7b03211" @default.
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