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- W2770052542 abstract "We report high-pressure magnetization and $^{35}$Cl NMR studies on $alpha$-RuCl$_3$ with pressure up to 1.5~GPa. At low pressures, the magnetic ordering is identified by both the magnetization data and the NMR data, where the $T_N$ shows a concave shape dependence with pressure. These data suggest stacking rearrangement along the $c$-axis. With increasing pressure, phase separation appears prominently at $Pge$~0.45~GPa, and the magnetic volume fraction is completely suppressed at $Pge$~1.05~GPa. Meanwhile, a phase-transition-like behavior emerges at high pressures in the remaining volume by a sharp drop of magnetization $M(T)$ upon cooling, with the transition temperature $T_x$ increased to ~250~K at 1~GPa. The $1/^{35}T_1$ is reduced by over three orders of magnitude when cooled below 100~K. This characterizes a high-pressure, low-temperature phase with nearly absent static susceptibility and low-energy spin fluctuations. The nature of the high-pressure ground state is discussed, where a magnetically disordered state is proposed as a candidate state." @default.
- W2770052542 created "2017-12-04" @default.
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- W2770052542 date "2017-11-27" @default.
- W2770052542 modified "2023-10-16" @default.
- W2770052542 title "High-pressure magnetization and NMR studies of <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mi>α</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>RuCl</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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- W2770052542 doi "https://doi.org/10.1103/physrevb.96.205147" @default.
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