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- W2770615449 abstract "Abstract Malonodinitrile, benzoylacetonitrile, and ethyl benzoylacetate were deprotonated in situ by nBuLi to give the reactive carbanions R2R3HC(−) (R2/R3 = CN/CN, CN/COPh, CO2Et/COPh), which nucleophilically attack the C N bond of the nitrilium clusters (Ph4P)[B10H9NCR1] (R1 = Me, Et). This reaction results in generation of push-pull alkenes bearing closo-decaborate clusters, [B10H9NHC(R1) CR2R3]2− (6 examples; up to 97% isolated yields). These species were isolated as the bis-tetraphenylposhphonium salts and were characterized by 1H and 11B NMR, HR ESI+/−-MS, and also by single-crystal X-ray diffraction." @default.
- W2770615449 created "2017-12-04" @default.
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- W2770615449 date "2018-02-01" @default.
- W2770615449 modified "2023-09-23" @default.
- W2770615449 title "Push-pull alkenes bearing closo-decaborate cluster generated via nucleophilic addition of carbanions to borylated nitrilium salts" @default.
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- W2770615449 doi "https://doi.org/10.1016/j.ica.2017.11.054" @default.
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