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- W2772023622 abstract "Abstract Plasmon‐driven catalysis has attracted great attention in recent years, but the reaction efficiency remains to be improved. Photothermal Fe 5 C 2 @Au core–shell nanostructures are fabricated through a self‐assembly process of Fe 5 C 2 and Au nanoparticles (NPs) with the assistance of hexanethiol, which can be highly efficient surface enhanced Raman spectroscopy (SERS) platforms for the study of plasmon‐driven dimerization of 4‐aminothiophenol (4‐ATP) and 4‐nitrothiophenol (4‐NTP). As compared to bare Au NPs, much accelerated reaction kinetics can be achieved on the Fe 5 C 2 @Au core–shell nanostructures by quantitatively determining the Raman intensity of the ν (N=N) band in the generated 4,4′‐dimercaptobenzene (DMAB). The photothermal effect from the Fe 5 C 2 NPs may lower the energy barrier and generate more hot electrons for the plasmon‐driven catalysis. This photothermal route may open up new avenues for enhancing the reaction rate and broadening the research area of the plasmon‐driven catalysis." @default.
- W2772023622 created "2017-12-22" @default.
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- W2772023622 date "2018-02-01" @default.
- W2772023622 modified "2023-09-24" @default.
- W2772023622 title "Photothermally Enhanced Plasmon-Driven Catalysis on Fe<sub>5</sub> C<sub>2</sub> @Au Core-Shell Nanostructures" @default.
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- W2772023622 doi "https://doi.org/10.1002/cctc.201701901" @default.
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