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• W2772027916 abstract "Highly N-doped nanoporous carbons have been of great interest as a high uptake CO2 adsorbent and as an efficient metal-free oxygen reduction reaction (ORR) catalyst. Therefore, it is essential to produce porosity-tunable and highly N-doped carbons through cost-effective means. Herein, we introduce the bioinspired synthesis of a monodisperse and N-enriched melaninlike polymer (MP) resembling the sepia biopolymer (SP) from oceanic cuttlefish. These polymers were subsequently utilized for highly N-doped synthetic carbon (MC) and biomass carbon (SC) spheres. An adequate CO2 activation process fine-tunes the ultramicroporosity (<1 nm) of N-doped MC and SC spheres, those with maximum ultramicroporosities of which show remarkable CO2 adsorption capacities. In addition, N-doped MC and SC with ultrahigh surface areas of 2677 and 2506 m2/g, respectively, showed excellent ORR activities with a favored four electron reduction pathway, long-term durability, and better methanol tolerance, comparable to a commercial Pt-based catalyst." @default.
• W2772027916 created "2017-12-22" @default.
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• W2772027916 date "2017-12-29" @default.
• W2772027916 modified "2023-09-23" @default.
• W2772027916 title "Bioinspired Synthesis of Melaninlike Nanoparticles for Highly N-Doped Carbons Utilized as Enhanced CO₂ Adsorbents and Efficient Oxygen Reduction Catalysts" @default.
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• W2772027916 doi "https://doi.org/10.1021/acssuschemeng.7b03680" @default.
• W2772027916 hasPublicationYear "2017" @default.
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