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- W2773642329 abstract "Replacement of oxygen evolution (OER) by the more readily oxidized urea is considered to be a promising strategy for electrocatalytic water-splitting. In this work, we report a FeOP film on nickel foam (FeOP/NF) via atomic layer deposition (ALD) of iron oxide and a subsequent phosphonation process, which acts as a superior bifunctional electrocatalyst for both urea evolution reaction (UOR) and hydrogen evolution reaction (HER). Benefiting from the synergetic effects, the FeOP/NF exhibits a low potential of 1.34 V (vs. RHE) at 10 mA cm−2 and a low Tafel slope of 57.2 mV dec−1 for UOR. Combined with the high HER activity of FeOP/NF, the urea-based overall water splitting can be performed with an low voltage of 1.43 V to deliver 10 mA cm−2 in 1.0 M KOH with 0.5 M urea, which is 200 mV lower than that for pure water splitting." @default.
- W2773642329 created "2017-12-22" @default.
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- W2773642329 date "2018-04-01" @default.
- W2773642329 modified "2023-10-16" @default.
- W2773642329 title "3D self-supported Fe O P film on nickel foam as a highly active bifunctional electrocatalyst for urea-assisted overall water splitting" @default.
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- W2773642329 doi "https://doi.org/10.1016/j.materresbull.2017.12.001" @default.
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