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- W2775498940 abstract "The design of cathodes for intercalation batteries requires consideration of both atomistic and electronic structure to facilitate redox at specific transition metal sites along with the concomitant diffusion of cations and electrons. Cation intercalation often brings about energy dissipative phase transformations that give rise to substantial intercalation gradients as well as multiscale phase and strain inhomogeneities. The layered α-V2O5 phase is considered to be a classical intercalation host but is plagued by sluggish diffusion kinetics and a series of intercalation-induced phase transitions that require considerable lattice distortion. Here, we demonstrate that a 1D tunnel-structured ζ-phase polymorph of V2O5 provides a stark study in contrast and can reversibly accommodate Li-ions without a large distortion of the structural framework and with substantial mitigation of polaronic confinement. Entirely homogeneous lithiation is evidenced across multiple cathode particles (in contrast to α-V2O5 partic..." @default.
- W2775498940 created "2017-12-22" @default.
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- W2775498940 date "2017-12-12" @default.
- W2775498940 modified "2023-10-15" @default.
- W2775498940 title "Mitigating Cation Diffusion Limitations and Intercalation-Induced Framework Transitions in a 1D Tunnel-Structured Polymorph of V<sub>2</sub>O<sub>5</sub>" @default.
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- W2775498940 doi "https://doi.org/10.1021/acs.chemmater.7b03800" @default.
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