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- W2777069969 abstract "A systematic study on the crystal structure and magnetic properties of GdCr1−xRuxO3 (where 0 ≤ x ≤ 0.15) was carried out by powder x-ray diffraction along with low temperature magnetization measurements. Lattice parameters and cell volume continuously increase with doping due to the incorporation and formation of higher ionic radius Ru4+ and Cr2+ ion, respectively. Pure GdCrO3 shows the antiferromagnetic (AFM) ordering at 170 K and a spin-reorientation transition around 8 K. Surprisingly, the AFM ordering temperature does not show any variation with the tetravalent Ru doping; while, spin-reorientation completely disappears with 5% Ru doping within the investigated temperature region. All these compounds exhibit magnetization reversal under low applied fields in field-cooled (FC) protocol. Highly delocalized 4d orbitals and occupation number of Ru4+ result in a decrease of antisymmetric exchange constant (D) with doping. Additionally, the formation of high-spin Cr2+ in weak octahedral field increases the effective magnetic moment for doped samples. Magnetic relaxation study in FC mode reveals the memory effect of pure GdCrO3. Magnetic field-assisted switching behavior study corroborates that magnetic state (positive or, negative) can easily be switched by the application of magnetic field." @default.
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- W2777069969 date "2018-03-01" @default.
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- W2777069969 title "Magnetization reversal, exchange interaction, and switching behavior studies on Ru doped GdCrO3" @default.
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- W2777069969 doi "https://doi.org/10.1016/j.jallcom.2017.12.222" @default.
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