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• W2777604326 abstract "Summary Bacteria can fabricate platinum group metal ( PGM ) catalysts cheaply, a key consideration of industrial processes and waste decontaminations. Biorecovery of PGM s from wastes is promising but PGM leachates made from metallic scraps are acidic. A two‐step biosynthesis ‘pre‐seeds’ metallic deposits onto bacterial cells benignly; chemical reduction of subsequent metal from acidic solution via the seeds makes bioscaffolded nanoparticles ( NP s). Cells of Escherichia coli were seeded using Pd( II ) or Pt( IV ) and exposed to a mixed Pd( II )/Pt( IV ) model solution under H 2 to make bimetallic catalyst. Its catalytic activity was assessed in the reduction of Cr( VI ), with 2 wt% or 5 wt% preloading of Pd giving the best catalytic activity, while 1 wt% seeds gave a poorer catalyst. Use of Pt seeds gave less effective catalyst in the final bimetallic catalyst, attributed to fewer and larger initial seeds as shown by electron microscopy, which also showed a different pattern of Pd and Pt deposition. Bimetallic catalyst (using cells preloaded with 2 wt% Pd) was used in the hydrogenation of soybean oil which was enhanced by ~fourfold using the bimetallic catalyst made from a model waste solution as compared to 2 wt% Pd preloaded cells alone, with a similar selectivity to cis C18:1 product as found using a Pd‐Al 2 O 3 commercial catalyst." @default.
• W2777604326 created "2018-01-05" @default.
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• W2777604326 date "2017-12-28" @default.
• W2777604326 modified "2023-10-16" @default.
• W2777604326 title "Biorefining of platinum group metals from model waste solutions into catalytically active bimetallic nanoparticles" @default.
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• W2777604326 doi "https://doi.org/10.1111/1751-7915.13030" @default.
• W2777604326 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5812250" @default.
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• W2777604326 hasPublicationYear "2017" @default.
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