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• W2778701150 startingPage "1131" @default.
• W2778701150 abstract "Tertiary phosphines remain widely utilized in synthesis, most notably as supporting ligands in metal complexes. A series of triarylphosphines bearing one to three hexa-peri-hexabenzocoronene (HBC) substituents has been prepared by an efficient divergent route. These superphenylphosphines, P{HBC(t-Bu)5}nPh3-n (n = 1-3), form the palladium complexes PdCl2L2 and Pd2Cl4L2 where the isomer distribution in solution is dependent on the number of HBC substituents. The crystalline structures of five complexes all show intramolecular π-stacking between HBC-phosphines to form a supramolecular bidentate-like ligand that distorts the metal coordination geometry. When n = 2 or 3, the additional HBC substituents engage in intermolecular π-stacking to assemble the complexes into continuous ribbons or sheets. The phosphines adopt HBC's characteristics including strong optical absorption, green emission, and redox activity." @default.
• W2778701150 created "2018-01-05" @default.
• W2778701150 creator A5066554992 @default.
• W2778701150 creator A5083995578 @default.
• W2778701150 creator A5091902040 @default.
• W2778701150 date "2018-01-09" @default.
• W2778701150 modified "2023-10-17" @default.
• W2778701150 title "Superphenylphosphines: Nanographene-Based Ligands That Control Coordination Geometry and Drive Supramolecular Assembly" @default.
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• W2778701150 doi "https://doi.org/10.1021/jacs.7b12251" @default.
• W2778701150 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29253338" @default.
• W2778701150 hasPublicationYear "2018" @default.
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