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• W2778903068 abstract "Polymer material properties are strongly affected by entanglement effects. For long polymer chains and composite materials, they are expected to be at the origin of many technically important phenomena, such as shear thinning or the Mullins effect, which microscopically can be related to topological constraints between chains. Starting from fully equilibrated highly entangled polymer melts, we investigate the effect of isochoric elongation on the entanglement structure and force distribution of such systems. Theoretically, the related viscoelastic response usually is discussed in terms of the tube model. We relate stress relaxation in the linear and nonlinear viscoelastic regimes to a primitive path analysis (PPA) and show that tension forces both along the original paths and along primitive paths, that is, the backbone of the tube, in the stretching direction correspond to each other. Unlike homogeneous relaxation along the chain contour, the PPA reveals a so far not observed long-lived clustering of topological constraints along the chains in the deformed state." @default.
• W2778903068 created "2018-01-05" @default.
• W2778903068 creator A5070039682 @default.
• W2778903068 creator A5078466092 @default.
• W2778903068 date "2017-12-29" @default.
• W2778903068 modified "2023-10-13" @default.
• W2778903068 title "Primitive Path Analysis and Stress Distribution in Highly Strained Macromolecules" @default.
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• W2778903068 doi "https://doi.org/10.1021/acsmacrolett.7b00808" @default.
• W2778903068 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5828704" @default.
• W2778903068 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29503762" @default.
• W2778903068 hasPublicationYear "2017" @default.
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